On-line Interrogation of Pebble Bed Reactor Fuel Using Passive Gamma-ray Spectometry

On-line Interrogation of Pebble Bed Reactor Fuel Using Passive Gamma-ray Spectometry
Title On-line Interrogation of Pebble Bed Reactor Fuel Using Passive Gamma-ray Spectometry PDF eBook
Author
Publisher
Pages
Release 2004
Genre
ISBN

Download On-line Interrogation of Pebble Bed Reactor Fuel Using Passive Gamma-ray Spectometry Book in PDF, Epub and Kindle

The Pebble Bed Reactor (PBR) is a helium-cooled, graphite-moderated high temperature nuclear power reactor. In addition to its inherently safe design, a unique feature of this reactor is its multipass fuel cycle in which graphite fuel pebbles (of varying enrichment) are randomly loaded and continuously circulated through the core until they reach their prescribed end-of-life burnup limit (8̃0,000-100,000 MWD/MTU). Unlike the situation with conventional light water reactors (LWRs), depending solely on computational methods to perform in-core fuel management will be highly inaccurate. As a result, an on-line measurement approach becomes the only accurate method to assess whether a particular pebble has reached its end-of-life burnup limit. In this work, an investigation was performed to assess the feasibility of passive gamma-ray spectrometry assay as an approach for on-line interrogation of PBR fuel for the simultaneous determination of burnup and enrichment on a pebble-by-pebble basis. Due to the unavailability of irradiated or fresh pebbles, Monte Carlo simulations were used to study the gamma-ray spectra of the PBR fuel at various levels of burnup. A pebble depletion calculation was performed using the ORIGEN code, which yielded the gamma-ray source term that was introduced into the input of an MCNP simulation. The MCNP simulation assumed the use of a high-purity coaxial germanium detector. Due to the lack of one-group high temperature reactor cross sections for ORIGEN, a heterogeneous MCNP model was developed to describe a typical PBR core. Subsequently, the code MONTEBURNS was used to couple the MCNP model and ORIGEN. This approach allowed the development of the burnup-dependent, one-group spectral-averaged PBR cross sections to be used in the ORIGEN pebble depletion calculation. Based on the above studies, a relative approach for performing the measurements was established. The approach is based on using the relative activities of Np-239/I-132 in combination with the relative activities of Cs-134/Co-60 (Co-60 is introduced as a dopant) to yield the burnup and enrichment for each pebble. Furthermore, a direct consequence of the relative approach is the ability to apply a self-calibration scheme using the multiple gamma lines of Ba-La-140 to establish the relative efficiency curve of the HPGe detector. An assessment of the expected uncertainty components in this approach showed that a maximum uncertainty of less than 5% should be feasible. To confirm the above findings, gamma-ray scans were performed on irradiated PULSTAR reactor fuel assemblies at North Carolina Sate University. The measurements used a 40% efficient n-type coaxial HPGe detector connected to an ORTEC DSPECplus digital Gamma-Ray Spectrometer, and a data acquisition computer.

Design and Construction of a Prototype Advanced On-line Fuel Burn-up Monitoring System for the Modular Pebble Bed Reactor

Design and Construction of a Prototype Advanced On-line Fuel Burn-up Monitoring System for the Modular Pebble Bed Reactor
Title Design and Construction of a Prototype Advanced On-line Fuel Burn-up Monitoring System for the Modular Pebble Bed Reactor PDF eBook
Author
Publisher
Pages
Release 2004
Genre
ISBN

Download Design and Construction of a Prototype Advanced On-line Fuel Burn-up Monitoring System for the Modular Pebble Bed Reactor Book in PDF, Epub and Kindle

Modular Pebble Bed Reactor (MPBR) is a high temperature gas-cooled nuclear power reactor currently under study as a next generation reactor system. In addition to its inherently safe design, a unique feature of this reactor is its multi-pass fuel circulation in which the fuel pebbles are randomly loaded and continuously cycled through the core until they reach their prescribed End-of-Life burn-up limit. Unlike the situation with a conventional light water reactor, depending solely on computational methods to perform in-core fuel management for MPBR will be highly inaccurate. An on-line measurement system is needed to accurately assess whether a given pebble has reached its End-of-Life burn-up limit and thereby provide an on-line, automated go/no-go decision on fuel disposition on a pebble-by-pebble basis. This project investigated approaches to analyzing fuel pebbles in real time using gamma spectroscopy and possibly using passive neutron counting of spontaneous fission neutrons to provide the speed, accuracy, and burn-up range required for burnup determination of MPBR. It involved all phases necessary to develop and construct a burn-up monitor, including a review of the design requirements of the system, identification of detection methodologies, modeling and development of potential designs, and finally, the construction and testing of an operational detector system. Based upon the research work performed in this project, the following conclusions are made. In terms of using gamma spectrometry, two possible approaches were identified for burnup assay. The first approach is based on the measurement of the absolute activity of Cs-137. However, due to spectral interference and the need for absolute calibration of the spectrometer, the uncertainty in burnup determination using this approach was found to range from (almost equal to) "40% at beginning of life to (almost equal to) "10% at the discharge burnup. An alternative approach is to use a relative burnup indicator. In this case, a self-calibration method was developed to obtain the spectrometer's relative efficiency curve based upon gamma lines emitted from 14°La. It was found that the ratio of 239Np/132I can be used in burnup measurement with an uncertainty of (almost equal to) "3% throughout the pebble's lifetime. In addition, by doping the fuel with 6°Co, the use of the 6°Co/134Cs and 239Np/132I ratios can simultaneously yield the enrichment and burnup of each pebble. A functional gamma-ray spectrometry measurement system was constructed and tested with light water reactor fuels. Experimental results were observed to be consistent with the predictions. On using the passive neutron counting method for the on-line burnup measurement, it was found that neutron emission rate of an irradiated pebble is sensitive to its burnup history and the spectral-averaged cross sections used in the depletion calculations; thus a large uncertainty exists in the correlation between neutron emission and burnup. At low burnup levels, the uncertainty in the neutron emission/burnup correlation is too high and neutron emission rate is too low so that it is impossible to determine a pebble's burnup by on-line neutron counting. At high burnup levels, due to the decreasing of the uncertainty in neutron emission rate and the super-linear feature of the correlation, the uncertainty in burnup determination was found to be (almost equal to)7% at the discharge burnup, which is acceptable for determining whether a pebble should be discharged or not. In terms of neutron detection, because an irradiated pebble is a weak neutron source and a much stronger gamma source, neutron detector system should have high neutron detection efficiency and strong gamma discrimination capability. Of all the commonly used neutron detectors, the He-3 and BF3 detector systems were found to be able to satisfy the requirement on detection efficiency; but their gamma discrimination capability is only marginal for this on-line application. Even with thick gamma shielding, these two types of detectors shall deteriorate in performance after a certain period of time of operation. Thus, two or more detector systems must be used alternatively for continuous measurement.

Investigation on Using Neutron Counting Techniques for Online Burnup Monitoring of Pebble Bed Reactor Fuels

Investigation on Using Neutron Counting Techniques for Online Burnup Monitoring of Pebble Bed Reactor Fuels
Title Investigation on Using Neutron Counting Techniques for Online Burnup Monitoring of Pebble Bed Reactor Fuels PDF eBook
Author
Publisher
Pages
Release 2004
Genre
ISBN

Download Investigation on Using Neutron Counting Techniques for Online Burnup Monitoring of Pebble Bed Reactor Fuels Book in PDF, Epub and Kindle

Modular Pebble Bed Reactor (MPBR) is a high temperature gas-cooled nuclear power reactor. In addition to its inherently safe design, a unique feature of this reactor is its multi-pass fuel circulation in which the fuel pebbles are randomly loaded and continuously cycled through the core until they reach their prescribed End-of-Life burnup limit. Unlike the situation with a conventional light water reactor, depending solely on computational methods to perform in-core fuel management for MPBR will be highly inaccurate. An on-line measurement system is needed to accurately assess whether a given pebble has reached its End-of-Life burnup limit and thereby provide an on-line, automated go/no-go decision on fuel disposition on a pebble-by-pebble basis. This project investigated the feasibility of using the passive neutron counting and active neutron/gamma counting for the on line fuel burnup measurement for MPBR. To investigate whether there is a correlation between neutron emission and fuel burnup, the MPBR fuel depletion was simulated under different irradiation conditions by ORIGEN2. It was found that the neutron emission from an irradiated pebble increases with burnup super-linearly and reaches to 10 4 neutron/sec/pebble at the discharge burnup. The photon emission from an irradiated pebble was found to be in the order of 10 13 photon/sec/pebble at all burnup levels. Analysis shows that the neutron emission rate of an irradiated pebble is sensitive to its burnup history and the spectral-averaged one-group cross sections used in the depletion calculations, which consequently leads to large uncertainty in the correlation between neutron emission and burnup. At low burnup levels, the uncertainty in the neutron emission/burnup correlation is too high and the neutron emission rate is too low so that it is impossible to determine a pebble2s burnup by on-line neutron counting at low burnup levels. At high burnup levels, the uncertainty in the neutron emission rate becomes less but is still large in quantity. However, considering the super-linear feature of the correlation, the uncertainty in burnup determination was found to be ̃7% at the discharge burnup, which is acceptable. Therefore, total neutron emission rate of a pebble can be used as a burnup indicator to determine whether a pebble should be discharged or not. The feasibility of using passive neutron counting methods for the on-line burnup measurement was investigated by using a general Monte Carlo code, MCNP, to assess the detectability of the neutron emission and the capability to discriminate gamma noise by commonly used neutron detectors. It was found that both He-3 and BF 3 detector systems are able to satisfy the requirement on detection efficiency; but their gamma discrimination capability is only marginal.

Dissertation Abstracts International

Dissertation Abstracts International
Title Dissertation Abstracts International PDF eBook
Author
Publisher
Pages 858
Release 2005
Genre Dissertations, Academic
ISBN

Download Dissertation Abstracts International Book in PDF, Epub and Kindle

Passive Nondestructive Assay of Nuclear Materials

Passive Nondestructive Assay of Nuclear Materials
Title Passive Nondestructive Assay of Nuclear Materials PDF eBook
Author Doug Reilly
Publisher
Pages 700
Release 1991
Genre Non-destructive testing
ISBN 9780160327247

Download Passive Nondestructive Assay of Nuclear Materials Book in PDF, Epub and Kindle

Liquid Life

Liquid Life
Title Liquid Life PDF eBook
Author Rachel Armstrong
Publisher
Pages 600
Release 2019
Genre
ISBN 9781950192182

Download Liquid Life Book in PDF, Epub and Kindle

If we lived in a liquid world, the concept of a "machine" would make no sense. Liquid life is metaphor and apparatus that discusses the consequences of thinking, working, and living through liquids. It is an irreducible, paradoxical, parallel, planetary-scale material condition, unevenly distributed spatially, but temporally continuous. It is what remains when logical explanations can no longer account for the experiences that we recognize as part of "being alive."Liquid Life references a third-millennial understanding of matter that seeks to restore the agency of the liquid soul for an ecological era, which has been banished by reductionist, "brute" materialist discourses and mechanical models of life. Offering an alternative worldview of the living realm through a "new materialist" and "liquid" study of matter, Armstrong conjures forth examples of creatures that do not obey mechanistic concepts like predictability, efficiency, and rationality. With the advent of molecular science, an increasingly persuasive ontology of liquid technologies can be identified. Through the lens of lifelike dynamic droplets, the agency for these systems exists at the interfaces between different fields of matter/energy that respond to highly local effects, with no need for a central organizing system.Liquid Life seeks an alternative partnership between humanity and the natural world. It provokes a re-invention of the languages of the living realm to open up alternative spaces for exploration, including contributor Rolf Hughes' "angelology" of language, which explores the transformative invocations of prose poetry, and Simone Ferracina's graphical notations that help shape our concepts of metabolism, upcycling, and designing with fluids. A conceptual and practical toolset for thinking and designing, liquid life reunites us with the irreducible "soul substance" of living things, which will neither be simply "solved," nor go away.

Springer Handbook of Mechanical Engineering

Springer Handbook of Mechanical Engineering
Title Springer Handbook of Mechanical Engineering PDF eBook
Author Karl-Heinrich Grote
Publisher Springer Nature
Pages 1310
Release 2020-12-09
Genre Technology & Engineering
ISBN 3030470350

Download Springer Handbook of Mechanical Engineering Book in PDF, Epub and Kindle

This resource covers all areas of interest for the practicing engineer as well as for the student at various levels and educational institutions. It features the work of authors from all over the world who have contributed their expertise and support the globally working engineer in finding a solution for today‘s mechanical engineering problems. Each subject is discussed in detail and supported by numerous figures and tables.