This textbook, based on the authors’ class-tested material, is accessible to students at the advanced undergraduate and graduate level in physics and engineering. While its primary function is didactic, this book’s comprehensive choice of topics and its clear and authoritative synthesis of ideas make it a useful reference for researchers, device engineers, and course instructors who wish to consolidate their knowledge of this field. The book takes the semi-classical approach where light is treated as a wave in accordance with the classical Maxwell equations, while matter is governed by quantum theory. It begins by introducing the postulates and mathematical framework of quantum theory, followed by the formalism of the density matrix which allows the transition from microscopic (quantum) quantities to macroscopic (classical) ones. Consequently, the equations describing the reaction of matter to the electromagnetic field in the form of polarization, magnetization, and current are derived. These equations (together with the Maxwell equations) form the complete system of equations sufficient to model a wide class of problems surrounding linear and nonlinear interactions of electromagnetic fields with matter. The nonlinear character of the governing equations determines parameters of the steady-state mode of the quantum generator and is also demonstrated in harmonic generation via propagation of laser radiation in various media. The touchstone description of magnetic phenomena will be of interest to scientists who deal with applications of magneto-resonance phenomena in biology and medicine. Other advanced topics covered include electric dipole transitions, magnetic dipole transitions, plasma transitions, and the devices that can be based on these and other electro-optical and nonlinear-optical systems. This textbook features numerous exercises, some of which are investigatory and some of which require computational solutions.

Since the early days of nonlinear optics in the 1960s, the field has expanded dramatically, and is now a vast and vibrant field with countless technological applications. Providing a gentle introduction to the principles of the subject, this textbook is ideal for graduate students starting their research in this exciting area. After basic ideas have been outlined, the book offers a thorough analysis of second harmonic generation and related second-order processes, before moving on to third-order effects, the nonlinear optics of short optical pulses and coherent effects such as electromagnetically-induced transparency. A simplified treatment of high harmonic generation is presented at the end. More advanced topics, such as the linear and nonlinear optics of crystals, the tensor nature of the nonlinear coefficients and their quantum mechanical representation, are confined to specialist chapters so that readers can focus on basic principles before tackling these more difficult aspects of the subject.

Introduction to Nonlinear Laser Spectroscopy focuses on the principles of nonlinear laser spectroscopy. This book discusses the experimental techniques of nonlinear optics and spectroscopy. Comprised of seven chapters, this book starts with an overview of the stimulated Raman effect and coherent anti-Stokes Raman spectroscopy, which can be used in a varied way to generate radiation in the ultraviolet and vacuum-ultraviolet areas. This text then explains the simplest quantum-mechanical system consisting of an isolated entity with energy eigenstates

This graduate-level textbook gives an introductory overview of the fundamentals of quantum nonlinear optics. It deals with the organization of radiation field, interaction between electronic system and radiation field, statistics of light, and mutual manipulation of light and matter. It also covers laser oscillation, dynamics of light, nonlinear optical response, and nonlinear spectroscopy, as well as ultrashort and ultrastrong laser pulse. In addition, latest results of the frontier of this science are presented. Problems and solutions help the reader to master and review the material.

Publisher Description

The quantum statistical properties of radiation represent an important branch of modern physics with rapidly increasing applications in spectroscopy, quantum generators of radiation, optical communication, etc. They have also an increasing role in fields other than pure physics, such as biophysics, psychophysics, biology, etc. The present monograph represents an extension and continuation of the previous monograph of this author entitled Coherence of Light (Van Nostrand Reinhold Company, London 1972, translated into Russian in the Publishing House Mir, Moscow 1974) and of a review chapter in Progress in Optics, Vol. 18 (E. Wolf (Ed.), North-Holland Publishing Company, Amsterdam 1980), published just recently. It applies the fundamental tools of the coherent-state technique, as described in Coherence of Light, to particular studies of the quantum statistical properties of radiation in its interaction with matter. In particular, nonlinear optical processes are considered, and purely quantum phenomena such as antibunching of photons are discussed. This book will be useful to research workers in the fields of quantum optics and electronics, quantum generators, optical communication and solid-state physics, as well as to students of physics, optical engineering and opto-electronics.