The embryonic development of femtoscience stems from advances made in the generation of ultrashort laser pulses. Beginning with mode-locking of glass lasers in the 1960s, the development of dye lasers brought the pulse width down from picoseconds to femtoseconds. The breakthrough in solid state laser pulse generation provided the current reliable table-top laser systems capable of average power of about 1 watt, and peak power density of easily watts per square centimeter, with pulse widths in the range of four to eight femtoseconds. Pulses with peak power density reaching watts per square centimeter have been achieved in laboratory settings and, more recently, pulses of sub-femtosecond duration have been successfully generated. As concepts and methodologies have evolved over the past two decades, the realm of ultrafast science has become vast and exciting and has impacted many areas of chemistry, biology and physics, and other fields such as materials science, electrical engineering, and optical communication. In molecular science the explosive growth of this research is for fundamental reasons. In femtochemistry and femtobiology chemical bonds form and break on the femtosecond time scale, and on this scale of time we can freeze the transition states at configurations never before seen. Even for n- reactive physical changes one is observing the most elementary of molecular processes. On a time scale shorter than the vibrational and rotational periods the ensemble behaves coherently as a single-molecule trajectory.

This is the second edition of this advanced textbook written for scientists who require further training in femtosecond science. Four years after pub- cation of the ?rst edition, femtosecond science has overcome new challenges and new application ?elds have become mature. It is necessary to take into account these new developments. Two main topics merged during this period that support important scienti?c activities: attosecond pulses are now gen- ated in the X-UV spectral domain, and coherent control of chemical events is now possible by tailoring the shape of femtosecond pulses. To update this advanced textbook, it was necessary to introduce these ?elds; two new ch- ters are in this second edition: “Coherent Control in Atoms, Molecules, and Solids”(Chap.11)and“AttosecondPulses”(Chap.12)withwell-documented references. Some changes, addenda, and new references are introduced in the ?rst edition’s ten original chapters to take into account new developments and updatethisadvancedtextbookwhichistheresultofascienti?cadventurethat started in 1991. At that time, the French Ministry of Education decided that, in view of the growing importance of ultrashort laser pulses for the national scienti?c community, a Femtosecond Centre should be created in France and devoted to the further education of scientists who use femtosecond pulses as a research tool and who are not specialists in lasers or even in optics.

Introduction to Laser Spectroscopy is a well-written, easy-to-read guide to understanding the fundamentals of lasers, experimental methods of modern laser spectroscopy and applications. It provides a solid grounding in the fundamentals of many aspects of laser physics, nonlinear optics, and molecular spectroscopy. In addition, by comprehensively combining theory and experimental techniques it explicates a variety of issues that are essential to understanding broad areas of physical, chemical and biological science. Topics include key laser types - gas, solid state, and semiconductor - as well as the rapidly evolving field of ultrashort laser phenomena for femtochemistry applications. The examples used are well researched and clearly presented. Introduction to Laser Spectroscopy is strongly recommended to newcomers as well as researchers in physics, engineering, chemistry and biology.* A comprehensive course that combines theory and practice* Includes a systematic and comprehensive description for key laser types* Written for students and professionals looking to gain a thorough understanding of modern laser spectroscopy

Femtosecond optics involves the study of ultra-short pulses of light. Understanding the behaviour of these light pulses makes it possible to develop ultra-fast lasers with a wide range of applications in such areas as medical imaging, chemical analysis and micro-machining. Written by two leading experts in the field, this book reviews the theory of the interaction of femtosecond light pulses with matter, femtosecond lasers and laser systems, and the principles of femtosecond coherent spectroscopy of impurity amorphous media. - reviews the theory of the interaction of femtosecond light pulses with matter - Discusses femtosecond lasers and laser systems - Considers the principles of femtosecond coherent spectroscopy of impurity amorphous media

Over the last few years, there has been a convergence between the fields of ultrafast science, nonlinear optics, optical frequency metrology, and precision laser spectroscopy. These fields have been developing largely independently since the birth of the laser, reaching remarkable levels of performance. On the ultrafast frontier, pulses of only a few cycles long have been produced, while in optical spectroscopy, the precision and resolution have reached one part in Although these two achievements appear to be completely disconnected, advances in nonlinear optics provided the essential link between them. The resulting convergence has enabled unprecedented advances in the control of the electric field of the pulses produced by femtosecond mode-locked lasers. The corresponding spectrum consists of a comb of sharp spectral lines with well-defined frequencies. These new techniques and capabilities are generally known as “femtosecond comb technology. ” They have had dramatic impact on the diverse fields of precision measurement and extreme nonlinear optical physics. The historical background for these developments is provided in the Foreword by two of the pioneers of laser spectroscopy, John Hall and Theodor Hänsch. Indeed the developments described in this book were foreshadowed by Hänsch’s early work in the 1970s when he used picosecond pulses to demonstrate the connection between the time and frequency domains in laser spectroscopy. This work complemented the advances in precision laser stabilization developed by Hall.

Keeping abreast of the latest techniques and applications, this new edition of the standard reference and graduate text on laser spectroscopy has been completely revised and expanded. While the general concept is unchanged, the new edition features a broad array of new material, e.g., ultrafast lasers (atto- and femtosecond lasers) and parametric oscillators, coherent matter waves, Doppler-free Fourier spectroscopy with optical frequency combs, interference spectroscopy, quantum optics, the interferometric detection of gravitational waves and still more applications in chemical analysis, medical diagnostics, and engineering.