Environmental Radionuclides presents a state-of-the-art summary of knowledge on the use of radionuclides to study processes and systems in the continental part of the Earth's environment. It is conceived as a companion to the two volumes of this series, which deal with isotopes as tracers in the marine environment (Livingston, Marine Radioactivity) and with the radioecology of natural and man-made terrestrial systems (Shaw, Radioactivity in Terrestrial Ecosystems). Although the book focuses on natural and anthropogenic radionuclides (radioactive isotopes), it also refers to stable environmental isotopes, which in a variety of applications, especially in hydrology and climatology, have to be consulted to evaluate radionuclide measurements in terms of the ages of groundwater and climate archives, respectively. The basic principles underlying the various applications of natural and anthropogenic radionuclides in environmental studies are described in the first part of the book. The book covers the two major groups of applications: the use of radionuclides as tracers for studying transport and mixing processes: and as time markers to address problems of the dynamics of such systems, manifested commonly as the so-called residence time in these systems. The applications range from atmospheric pollution studies, via water resource assessments to contributions to global climate change investigation. The third part of the book addresses new challenges in the development of new methodological approaches, including analytical methods and fields of applications. - A state-of-the-art summary of knowledge on the use of radionuclides - Conceived as a companion to the two volumes of this series, which deal with isotopes as tracers

This book provides extensive and comprehensive information to researchers and academicians who are interested in radionuclide contamination, its sources and environmental impact. It is also useful for graduate and undergraduate students specializing in radioactive-waste disposal and its impact on natural as well as manmade environments. A number of sites are affected by large legacies of waste from the mining and processing of radioactive minerals. Over recent decades, several hundred radioactive isotopes (radioisotopes) of natural elements have been produced artificially, including 90Sr, 137Cs and 131I. Several other anthropogenic radioactive elements have also been produced in large quantities, for example technetium, neptunium, plutonium and americium, although plutonium does occur naturally in trace amounts in uranium ores. The deposition of radionuclides on vegetation and soil, as well as the uptake from polluted aquifers (root uptake or irrigation) are the initial point for their transfer into the terrestrial environment and into food chains. There are two principal deposition processes for the removal of pollutants from the atmosphere: dry deposition is the direct transfer through absorption of gases and particles by natural surfaces, such as vegetation, whereas showery or wet deposition is the transport of a substance from the atmosphere to the ground by snow, hail or rain. Once deposited on any vegetation, radionuclides are removed from plants by the airstre am and rain, either through percolation or by cuticular scratch. The increase in biomass during plant growth does not cause a loss of activity, but it does lead to a decrease in activity concentration due to effective dilution. There is also systemic transport (translocation) of radionuclides within the plant subsequent to foliar uptake, leading the transfer of chemical components to other parts of the plant that have not been contaminated directly.

The 3-volume set highlights the behavior of radionuclides in the environment and focusing on the development of related fields of study, including microbiology and nanoscience. In this context, it discusses the behavior of radionuclides released in areas of Lake Karachai in Ural, and those released as a result of Chernobyl accident (1986), and in Fukushima (2011). Volume I presents the experiences gained in South Urals (“Mayak” plant, Lake Karachai), providing a scientific basis for more precise understanding of the behavior of radionuclides in complex subsurface environments. On the basis of monitoring data, it examines the pathways of radionuclide migration and the influence of the geological environment and groundwater on the migration, with a particular focus on particles from the nanoscale to microscale. It also discusses the function of microbes and microscale particles, from their direct interaction with radionuclides to their ecological role in changing the physic-chemical condition of a given environment. Lastly, the protective properties of geological media are also characterized, and mathematical modeling of contaminant migration in the area of Lake Karachai is used to provide information regarding the migration of radionuclides.

This book, the third in the series Behavior of Radionuclides in the Environment, is dedicated to Fukushima. Major findings from research since 2011 are reviewed concerning the behavior of radionuclides released into the environment due to the Fukushima Dai-ichi Nuclear Power Plant accident, including atmospheric transport and fallout of radionuclides, their fate, and transport in the soil-water environment, behavior in freshwater, coastal and marine environment, transfer in the terrestrial and agricultural environment. Volume III discusses not only radionuclides dynamics in the environment in the short- and mid-term, but also modeling and prediction of long-term time changes. Along with reviews, the book contains original data and results not published previously. It was spearheaded by the authors from the Institute of Environmental Radioactivity at Fukushima University, established two years after the Fukushima accident, with their collaborators from Japan, Russia, and Ukraine. The knowledge emerging from the studies of the environmental behavior of Fukushima-derived radionuclides enables us to move forward in understanding mechanisms of environmental contamination and leads to better modeling and prediction of long-term pollution effects in general.

Radioactive particles have been released to the environment from a number of sources, including nuclear weapon tests, nuclear accidents and discharges from nuclear installations. Particle characteristics influence the mobility, biological uptake and effects of radionuclides, hence information on these characteristics is essential for assessing environmental impact and risks. This publication presents a series of papers covering sources and source term characterisation, methodologies for characterizing particles, and the impact of particles on the behaviour of radioactive particles in the environment. Sources covered include the Chernobyl accident, nuclear weapons accidents at Thule and Palomares accident, the discharges from Dounreay and Krashnoyarsk, and depleted uranium in Kosovo and Kuwait. The overall aim is that an increased understanding of particle characteristics and behavior will help to reduce some of the uncertainties in environmental impact and risk assessment for particle contaminated areas.

Nuclear sites become contaminated with radionuclides due to accidents and activities carried out without due consideration for the environment. Naturally-occurring radioactive materials (NORM) released by industrial processes such as coal power production and fertilizer manufacture may also require clean-up. Environmental remediation and restoration aim to reduce exposure to radiation from contaminated soil or groundwater. This book provides a comprehensive overview of this area. Part 1 provides an introduction to the different types of contaminated site and their characteristics. Part 2 addresses environmental restoration frameworks and processes. Part 3 then reviews different remediation techniques and methods of waste disposal. - Explores types and characteristics of contaminated nuclear and NORM sites - Provides an in depth guide to environmental restoration frameworks and processes including stakeholder involvement, risk assessment and cost-benefit analysis in the remediation and restoration of contaminated nuclear and NORM sites - Offers coverage of remediation techniques and waste disposal from electrokinetic remediation to in situ and ex situ bioremediation of radionuclides contaminated soils

Cosmogenic radionuclides are radioactive isotopes which are produced by natural processes and distributed within the Earth system. With a holistic view of the environment the authors show in this book how cosmogenic radionuclides can be used to trace and to reconstruct the history of a large variety of processes. They discuss the way in which cosmogenic radionuclides can assist in the quantification of complex processes in the present-day environment. The book aims to demonstrate to the reader the strength of analytic tools based on cosmogenic radionuclides, their contribution to almost any field of modern science, and how these tools may assist in the solution of many present and future problems that we face here on Earth. The book provides a comprehensive discussion of the basic principles behind the applications of cosmogenic (and other) radionuclides as environmental tracers and dating tools. The second section of the book discusses in some detail the production of radionuclides by cosmic radiation, their transport and distribution in the atmosphere and the hydrosphere, their storage in natural archives, and how they are measured. The third section of the book presents a number of examples selected to illustrate typical tracer and dating applications in a number of different spheres (atmosphere, hydrosphere, geosphere, biosphere, solar physics and astronomy). At the same time the authors have outlined the limitations of the use of cosmogenic radionuclides. Written on a level understandable by graduate students without specialist skills in physics or mathematics, the book addresses a wide audience, ranging from archaeology, biophysics, and geophysics, to atmospheric physics, hydrology, astrophysics and space science.