The papers collected in this volume in honor of the late Stanisław Kielich cover an impressive range of modern subjects in molecular science. These subjects include, among others, the nonlinear optics of molecules, new approaches to the electronic structure of large molecules, the properties of carbon nanotubes, fluorescence polarization spectroscopy, computational studies of systems of fundamental interest to collision-induced spectroscopy, the simulation of fluids, NLO materials, chemical bonding in complex molecules, the NLO properties of functionalized DNA and the magnetic properties of molecular assemblies. Written by eminent specialists, the papers should offer valuable guidance to a wide community of graduate students and researchers.

Laser physics and nonlinear optics are fields which have been intimately con nected from their beginning. Nonlinear optical effects such as second-har monic generation fulfil vital functions in many laser systems. Conversely advances in laser development quickly lead to progress in nonlinear optics. Of particular importance has been the development of tunable visible and uv lasers. With the ability to tune the laser frequency into close resonance with atomic transition frequencies, one can produce a large resonance en hancement of the nonlinearity. This permits the observation of a great var iety of nonlinear optical processes in dilute media such as atomic vapours. In recent years much of the research effort in nonlinear optics has been directed towards the use of such media, and it is this area which forms the subject of the present book. We review a wide range of nonlinear optical processes in atomic vapours, molecular gases and cryogenic liquids. At the same time we have tried to treat the subject in sufficient depth to be useful to research workers in the field. To achieve this, a measure of selectivity has been introduced by emphasising those nonlinear processes which are seen to have applications as sources of tunable coherent radiation. Thus we have not discussed in any detail those nonlinear processes whose main applications are in spec troscopy, such as Doppler-free two-photon absorption.

Contemporary Nonlinear Optics discusses the different activities in the field of nonlinear optics. The book is comprised of 10 chapters. Chapter 1 presents a description of the field of nonlinear guided-wave optics. Chapter 2 surveys a new branch of nonlinear optics under the heading optical solitons. Chapter 3 reviews recent progress in the field of optical phase conjugation. Chapter 4 discusses ultrafast nonlinear optics, a field that is growing rapidly with the ability of generating and controlling femtosecond optical pulses. Chapter 5 examines a branch of nonlinear optics that may be termed nonlinear quantum optics. Chapter 6 reviews the new field of photorefractive adaptive neural networks. Chapter 7 presents a discussion of recent successes in the development of nonlinear optical media based on organic materials. Chapter 8 reviews the field of nonlinear optics in quantum confined structures. Chapter 9 reviews the field of nonlinear laser spectroscopy, with emphasis on advances made during the 1980s. Finally, Chapter 10 reviews the field of nonlinear optical dynamics by considering nonlinear optical systems that exhibit temporal, spatial, or spatio-temporal instabilities. This book is a valuable source for physicists and other scientists interested in optical systems and neural networks.

This book draws together the principal ideas that form the basis of atomic, molecular, and optical science and engineering. It covers the basics of atoms, diatomic molecules, atoms and molecules in static and electromagnetic fields and nonlinear optics. Exercises and bibliographies supplement each chapter, while several appendices present such important background information as physics and math definitions, atomic and molecular data, and tensor algebra. Accessible to advanced undergraduates, graduate students, or researchers who have been trained in one of the conventional curricula of physics, chemistry, or engineering but who need to acquire familiarity with adjacent areas in order to pursue their research goals.

This is the first volume of textbooks on atomic, molecular and optical physics, aiming at a comprehensive presentation of this highly productive branch of modern physics as an indispensable basis for many areas in physics and chemistry as well as in state of the art bio- and material-sciences. It primarily addresses advanced students (including PhD students), but in a number of selected subject areas the reader is lead up to the frontiers of present research. Thus even the active scientist is addressed. This volume 1 provides the canonical knowledge in atomic physics together with basics of modern spectroscopy. Starting from the fundamentals of quantum physics, the reader is familiarized in well structured chapters step by step with the most important phenomena, models and measuring techniques. The emphasis is always on the experiment and its interpretation, while the necessary theory is introduced from this perspective in a compact and occasionally somewhat heuristic manner, easy to follow even for beginners.

Laser physics and nonlinear optics are fields which have been intimately con nected from their beginning. Nonlinear optical effects such as second-har monic generation fulfil vital functions in many laser systems. Conversely advances in laser development quickly lead to progress in nonlinear optics. Of particular importance has been the development of tunable visible and uv lasers. With the ability to tune the laser frequency into close resonance with atomic transition frequencies, one can produce a large resonance en hancement of the nonlinearity. This permits the observation of a great var iety of nonlinear optical processes in dilute media such as atomic vapours. In recent years much of the research effort in nonlinear optics has been directed towards the use of such media, and it is this area which forms the subject of the present book. We review a wide range of nonlinear optical processes in atomic vapours, molecular gases and cryogenic liquids. At the same time we have tried to treat the subject in sufficient depth to be useful to research workers in the field. To achieve this, a measure of selectivity has been introduced by emphasising those nonlinear processes which are seen to have applications as sources of tunable coherent radiation. Thus we have not discussed in any detail those nonlinear processes whose main applications are in spec troscopy, such as Doppler-free two-photon absorption.