This book studies the dynamics of fundamental collective excitations in quantum materials, focusing on the use of state-of-the-art ultrafast broadband optical spectroscopy. Collective behaviour in solids lies at the origin of several cooperative phenomena that can lead to profound transformations, instabilities and phase transitions. Revealing the dynamics of collective excitations is a topic of pivotal importance in contemporary condensed matter physics, as it provides information on the strength and spatial distribution of interactions and correlation. The experimental framework explored in this book relies on setting a material out-of-equilibrium by an ultrashort laser pulse and monitoring the photo-induced changes in its optical properties over a broad spectral region in the visible or deep-ultraviolet. Collective excitations (e.g. plasmons, excitons, phonons...) emerge either in the frequency domain as spectral features across the probed range, or in the time domain as coherent modes triggered by the pump pulse. Mapping the temporal evolution of these collective excitations provides access to the hierarchy of low-energy phenomena occurring in the solid during its path towards thermodynamic equilibrium. This methodology is used to investigate a number of strongly interacting and correlated materials with an increasing degree of internal complexity beyond conventional band theory.

Mots-clés de l'auteur: Ultrafast Optical Spectroscopy ; Many-Body Physics ; Collective Excitations ; Strongly Correlated Electron Systems.

This book advances understanding of light-induced phase transitions and nonequilibrium orders that occur in a broken-symmetry system. Upon excitation with an intense laser pulse, materials can undergo a nonthermal transition through pathways different from those in equilibrium. The mechanism underlying these photoinduced phase transitions has long been researched, but many details in this ultrafast, non-adiabatic regime still remain to be clarified. The work in this book reveals new insights into this phenomena via investigation of photoinduced melting and recovery of charge density waves (CDWs). Using several time-resolved diffraction and spectroscopic techniques, the author shows that the light-induced melting of a CDW is characterized by dynamical slowing-down, while the restoration of the symmetry-breaking order features two distinct timescales: A fast recovery of the CDW amplitude is followed by a slower re-establishment of phase coherence, the latter of which is dictated by the presence of topological defects in the CDW. Furthermore, after the suppression of the original CDW by photoexcitation, a different, competing CDW transiently emerges, illustrating how a hidden order in equilibrium can be unleashed by a laser pulse. These insights into CDW systems may be carried over to other broken-symmetry states, such as superconductivity and magnetic ordering, bringing us one step closer towards manipulating phases of matter using a laser pulse.

The 1995 observation of Bose-Einstein condensation in dilute atomic vapours spawned the field of ultracold, degenerate quantum gases. Unprecedented developments in experimental design and precision control have led to quantum gases becoming the preferred playground for designer quantum many-body systems.This self-contained volume provides a broad overview of the principal theoretical techniques applied to non-equilibrium and finite temperature quantum gases. Covering Bose-Einstein condensates, degenerate Fermi gases, and the more recently realised exciton-polariton condensates, it fills a gap by linking between different methods with origins in condensed matter physics, quantum field theory, quantum optics, atomic physics, and statistical mechanics. Thematically organised chapters on different methodologies, contributed by key researchers using a unified notation, provide the first integrated view of the relative merits of individual approaches, aided by pertinent introductory chapters and the guidance of editorial notes.Both graduate students and established researchers wishing to understand the state of the art will greatly benefit from this comprehensive and up-to-date review of non-equilibrium and finite temperature techniques in the exciting and expanding field of quantum gases and liquids./a

This thesis explores the physics of non-equilibrium quantum dynamics in homogeneous two-dimensional (2D) quantum gases. Ultracold quantum gases driven out of equilibrium have been prominent platforms for studying quantum many-body physics. However, probing non-equilibrium dynamics in conventionally trapped, inhomogeneous atomic quantum gases has been a challenging task because coexisting mass transport and spreading of quantum correlations often complicate experimental analyses. In this work, the author solves this technical hurdle by producing ultracold cesium atoms in a quasi-2D optical box potential. The exquisite optical trap allows one to remove density inhomogeneity in a degenerate quantum gas and control its dimensionality. The author also details the development of a high-resolution, in situ imaging technique to monitor the evolution of collective excitations and quantum transport down to atomic shot-noise, and at the length scale of elementary collective excitations. Meanwhile, tunable Feshbach resonances in ultracold cesium atoms permit precise and dynamical control of interactions with high temporal and even spatial resolutions. By employing these state-of-the-art techniques, the author performed interaction quenches to control the generation and evolution of quasiparticles in quantum gases, presenting the first direct measurement of quantum entanglement between interaction quench generated quasiparticle pairs in an atomic superfluid. Quenching to attractive interactions, this work shows stimulated emission of quasiparticles, leading to amplified density waves and fragmentation, forming 2D matter-wave Townes solitons that were previously considered impossible to form in equilibrium due to their instability. This thesis unveils a set of scale-invariant and universal quench dynamics and provides unprecedented tools to explore quantum entanglement transport in a homogenous quantum gas.