Optical frequency combs (OFC) have revolutionized various applications in applied and fundamental sciences that rely on the determination of absolute optical frequencies and frequency differences. The latter requires only stabilization of the spectral distance between the individual comb lines of the OFC, allowing to tailor and reduce system complexity of the OFC generator (OFCG). One such application is the quantum test of the universality of free fall within the QUANTUS experimental series. Within the test, the rate of free fall of two atomic species, Rb and K, in micro-gravity will be compared. The aim of this thesis was the development of a highly compact, robust, and space-suitable diode laser-based OFCG with a mode-locked optical spectrum in the wavelength range around 780 nm. A diode laser-based OFCG was developed, which exceeds the requirements with a spectral bandwidth > 16 nm at 20 dBc, a comb line optical power > 650 nW (at 20 dBc), a pulse repetition rate of 3.4 GHz, and an RF linewidth of the free-running pulse repetition rate < 10 kHz. To realize a proof-of-concept demonstrator module, the diode laser-based OFCG was hybrid-integrated into a space-suitable technology platform that has been developed for future QUANTUS experiments. Proof of sufficient RF stability of the OFCG was provided by stabilizing the pulse repetition rate to an external RF reference. This resulted in a stabilized pulse repetition rate with an RF linewidth smaller than 1.4 Hz (resolution limited), thus exceeding the requirement. The developed diode laser-based OFCG represents an important step towards an improved comparison of the rate of free fall of Rb and K quantum gases within the QUANTUS experiments in micro-gravity.

Over the last few years, there has been a convergence between the fields of ultrafast science, nonlinear optics, optical frequency metrology, and precision laser spectroscopy. These fields have been developing largely independently since the birth of the laser, reaching remarkable levels of performance. On the ultrafast frontier, pulses of only a few cycles long have been produced, while in optical spectroscopy, the precision and resolution have reached one part in Although these two achievements appear to be completely disconnected, advances in nonlinear optics provided the essential link between them. The resulting convergence has enabled unprecedented advances in the control of the electric field of the pulses produced by femtosecond mode-locked lasers. The corresponding spectrum consists of a comb of sharp spectral lines with well-defined frequencies. These new techniques and capabilities are generally known as “femtosecond comb technology. ” They have had dramatic impact on the diverse fields of precision measurement and extreme nonlinear optical physics. The historical background for these developments is provided in the Foreword by two of the pioneers of laser spectroscopy, John Hall and Theodor Hänsch. Indeed the developments described in this book were foreshadowed by Hänsch’s early work in the 1970s when he used picosecond pulses to demonstrate the connection between the time and frequency domains in laser spectroscopy. This work complemented the advances in precision laser stabilization developed by Hall.